//Instantiating a Workbook object
Workbook workbook = new Workbook();
//Obtaining the reference of the first (default) worksheet by passing its sheet index
Worksheet worksheet = workbook.Worksheets[0];
//Accessing the "A1" cell from the worksheet
Aspose.Cells.Cell cell = worksheet.Cells["A1"];
//Adding some value to the "A1" cell
cell.PutValue("Visit Aspose!");
//Create a style object
Style style = cell.GetStyle();
//Setting the line style of the top border
style.Borders[BorderType.TopBorder].LineStyle = CellBorderType.Thick;
//Setting the color of the top border
style.Borders[BorderType.TopBorder].Color = Color.Black;
//Setting the line style of the bottom border
style.Borders[BorderType.BottomBorder].LineStyle = CellBorderType.Thick;
//Setting the color of the bottom border
style.Borders[BorderType.BottomBorder].Color = Color.Black;
//Setting the line style of the left border
style.Borders[BorderType.LeftBorder].LineStyle = CellBorderType.Thick;
//Setting the color of the left border
style.Borders[BorderType.LeftBorder].Color = Color.Black;
//Setting the line style of the right border
style.Borders[BorderType.RightBorder].LineStyle = CellBorderType.Thick;
//Setting the color of the right border
style.Borders[BorderType.RightBorder].Color = Color.Black;
//Apply the border styles to the cell
cell.SetStyle(style);
//Saving the Excel file
workbook.Save("C:\\book1.xls");
信息来自: http://www.aspose.com/documentation/.net-components/aspose.cells-for-.net/adding-borders-to-cells.html