Customize AE toolbar

//Create UID's and add new items to the ToolBarControl
            UID uID = new UIDClass();
            uID.Value = "esriControlCommands.ControlsOpenDocCommand";
            axToolbarControl1.AddItem(uID, 0, -1, false, -1, esriCommandStyles.esriCommandStyleIconOnly);

            uID.Value = "esriControlCommands.ControlsMapZoomInTool";
            axToolbarControl1.AddItem(uID, -1, -1, true, -1, esriCommandStyles.esriCommandStyleIconAndText);

            uID.Value = "esriControlCommands.ControlsMapZoomOutTool";
            axToolbarControl1.AddItem(uID, -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);

            uID.Value = "esriControlCommands.ControlsMapPanTool";
            axToolbarControl1.AddItem(uID, -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);

            uID.Value = "esriControlCommands.ControlsMapFullExtentCommand";
            axToolbarControl1.AddItem(uID, -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);

            uID.Value = "esriControlCommands.ControlsMapZoomToLastExtentBackCommand";
            axToolbarControl1.AddItem(uID, -1, -1, true, 20, esriCommandStyles.esriCommandStyleTextOnly);

            uID.Value = "esriControlCommands.ControlsMapZoomToLastExtentForwardCommand";
            axToolbarControl1.AddItem(uID, -1, -1, false, -1, esriCommandStyles.esriCommandStyleTextOnly);
 

or

//Add items to the ToolbarControls
        axToolbarControl1.AddItem("esriControlCommands.ControlsOpenDocCommand", -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconOnly);
        axToolbarControl1.AddItem("esriControlCommands.ControlsMapZoomInTool", -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);
        axToolbarControl1.AddItem("esriControlCommands.ControlsMapZoomOutTool", -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);
        axToolbarControl1.AddItem("esriControlCommands.ControlsMapPanTool", -1, -1, false, -1, esriCommandStyles.esriCommandStyleIconAndText);