signature=198a3932ef965ede5acb628df4f8cada,Signatures of the spin-phonon coupling in Fe1+yTe1-xSex a...

摘要:

Raman scattering spectra of FeTeSe(x=0, y=0.07; x=0.1, y=0.05 and x=0.4, y=0.02) alloys are measured in a temperature range between 20 K and 300 K. The A1g and B1g Raman active modes have been experimentally observed at energies 156 and 198 cm, which is in rather good agreement with the lattice dynamics calculation. The antiferromagnetic spin ordering below 70 K in FeTe leaves a fingerprint only in the Bphonon mode linewidth and energy, whose temperature dependence follows the normalized magnetic susceptibility, indicating the presence of the spin-phonon coupling. The frequency and the linewidth of the Amode assume a conventional anharmonic temperature dependence in all measured samples, which is also the case for the Bmode in the Se doped samples. The linewidth (energy) of the Amode decreases (increases) with doping, whereas the opposite is seen for the Bmode.

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